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    Binational survey of personal protective equipment (PPE) pollution driven by the COVID-19 pandemic in coastal environments: abundance, distribution, and analytical characterization
    (Elsevier, 2021-12-11)
    In the present contribution, two nationwide surveys of personal protective equipment (PPE) pollution were conducted in Peru and Argentina aiming to provide valuable information regarding the abundance and distribution of PPE in coastal sites. Additionally, PPE items were recovered from the environment and analyzed by Fourier transformed infrared (FTIR) spectroscopy, Scanning electron microscopy (SEM) with Energy dispersive X-ray (EDX), and X-ray diffraction (XRD), and compared to brand-new PPE in order to investigate the chemical and structural degradation of PPE in the environment. PPE density (PPE m−2) found in both countries were comparable to previous studies. FTIR analysis revealed multiple polymer types comprising common PPE, mainly polypropylene, polyamide, polyethylene terephthalate, and polyester. SEM micrographs showed clear weathering signs, such as cracks, cavities, and rough surfaces in face masks and gloves. EDX elemental mapping revealed the presence of elemental additives, such as Ca in gloves and face masks and AgNPs as an antimicrobial agent. Other metals found on the surface of PPE were Mo, P, Ti, and Zn. XRD patterns displayed a notorious decrease in the crystallinity of polypropylene face masks, which could alter its interaction with external contaminants and stability. The next steps in this line of research were discussed.
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    Consideration of Plastic Emissions in Life Cycle Assessments
    (Springer International Publishing, 2025-01-01)
    Life cycle assessment (LCA) is the method most frequently used to systematically assess the environmental impacts of products and services over their entire life cycle. Several environmental impacts, such as global warming or ozone depletion, are covered. Life cycle assessments do not yet allow, however, for considering the consequences of plastic waste leaking into the environment. Thus, plastic products such as PET bottles might appear beneficial (having, for example, a lower carbon footprint than alternatives such as glass bottles) although they contribute to potentially harmful effects if released into the environment. In addition, the absence of an impact assessment method addressing plastic emissions limits the possibility of analyzing the trade-offs between impact categories. In order to provide an overview of the state of the art of plastic emissions in LCA, the chapter begins with an overview of the LCA methodology in general. There follows a description of the potential impact pathways of plastic emissions using a framework developed by the International Working Group MarILCA on Marine Impacts in Life Cycle Assessment. Within the framework, relevant existing impact categories are discussed, and new ones are proposed. The following section describes accounting methods for plastic emissions and ways of defining plastic flows in life cycle inventory (LCI). The already developed approaches addressing plastic emissions in life cycle impact assessment (LCIA) are then described in relation to the framework and, in addition, examples of applications (case studies) are presented. Finally, future research needs are discussed.
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